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- Innovative particleboard material from the organic fraction of municipal solid wastePublication . Santos, Michael M.; Diez, Maria Antonia; Suárez, Marta; Centeno, Teresa A.This study presents a challenging approach that addresses the efficient management of the organic fraction of municipal solid waste (OFMSW) by hydrothermal carbonization (HTC) for the development of novel sustainable low-CO2 building materials. Mild HTC treatment at 180 °C for 2 h transformed low-grade OFMSW into a renewable carbonaceous solid (hydrochar), which displays promising properties for application in particleboards. Taking advantage of the presence of extractives acting as natural binders, the hydrochar particles with sizes of <0.3 mm, 0.3–1 mm, and 1–2 mm agglomerate successfully by simple pressing at 3 MPa for 7 min at room temperature (∼ 25 °C). The resulting binderless monolithic probes display a density of 838 and 883 kg/m3 for the finest and coarsest grain sizes, respectively, and approximately 30% porosity. The mechanical resistance is enhanced by the use of larger particle sizes, and values of modulus of rupture and tensile strength of 21.64 MPa and 18.99 MPa are reached, respectively. The thermal conductivity of the probes in the range of 0.091–0.132 W/(m∙K) suggests the potential of OFMSW-derived hydrochar for thermal insulation panels.
- Reducing cement consumption in mortars by waste-derived hydrocharsPublication . Santos, Michael M.; Marques Sierra, Antonio Luis; Amado Fierro, Álvaro; Suárez, Marta; Blanco, Francisco A.; González La Fuente, José Manuel; Diez, Maria Antonia; Centeno, Teresa A.Waste-derived hydrochars are presented for the first time as promising materials to reduce the consumption of natural resources and the carbon footprint of the cement industry, while eliminating waste and sequestering a high amount of carbon in civil infrastructures. Rice husk (RH) and stabilized organic waste from a mixed municipal waste mechanical-biological treatment plant (SOW) were subjected to hydrothermal carbonization at 200 °C for 2 h and the resulting hydrochars were thoroughly evaluated as cement substitutes in fresh and hardened mortars. Compared to the control, mortars with 1.25–5 wt% of cement replaced by hydrochar from stabilized organic fraction caused a decrease in compressive strength of about 50–60% at 28 days of curing, while flexural strength was diminished by about 38–47%. The use of rice husk-derived hydrochar led to a reduction of 32–47% in compressive strength and of 22–34% in flexural strength. With compressive and flexural strengths of 27–41 and 3.31–4.92 MPa, respectively, blended mortars (28 days) display good prospects for use in plastering, rendering, masonry, partition panels and low-load paving. On the other hand, substituting 5 wt% of cement by hydrochar decreases the thermal conductivity and increases electrical resistivity of the mortar by 25–30%, which enhances thermal insulation properties and potential durability. This approach opens a new avenue for large-scale application of biowaste hydrochars as secondary raw materials for sustainable construction.